To smoke weed/pot/ganja and get high.
The magic dragon usually refers to the item the marijuana is being smoked in. ie- bong, joint, pipe
A bunch of friends are sitting around a campfire and about to smoke. John pulls out his pipe and bag of weed and says to the whole group " Who wants to puff the magic dragon?"
Duke William and Dutchess Kate puffed the magic dragon on their wedding night and got baked off their royal asses.
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