to masturbate while fantasizing about having sex with Smurfette.
"Man, Smurfette was lookin so good on Saturday morning's episode...I just HAD to smurf off!"
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Is when the person who started the smurf off, usually a Squeeb, throws a little blue man at you and runs away laughing an evil laugh.
"Ahhh.. Smurf off.. Mandy" .. Runs away " muahha hahaha"
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