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Very small left-over particles of marijuana.
Grunyuns are created from the process of breaking down buds, rolling joints or blunts, or packing pipes & bongs.
The term shake is a comparable synonym.
"Dude don't throw that out! You know i save all the grunyuns!"
"If I want to smoke bad enough, I scrape together all the grunyuns I can find"
"Ehhh BOBO!! lemme get them grunyuns when you get done rolling that blunt!
The crumbs of chips and flavoring at the bottom of a bag of chips.
Hey man, you gonna eat those grunyuns?